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Light‐triggered chemical fuel generation from photolytic fuel‐carrier molecules. (a) Design and photolytic mechanism of fuel‐carrier molecules, ONB‐HFIP, which undergo UV‐triggered photolysis to release HFIP fuel and reaction byproducts. (b) Color change of ONB‐HFIP in solution as a function of UV irradiation time. (c) Time‐resolved <t>HPLC</t> chromatograms and (d) UV‐vis absorption spectra of ONB‐HFIP in solution as a function of UV irradiation time. (e) Conversion degree of photolytic reaction, estimated from the changing ratio of HPLC peak areas and UV‐vis absorption intensities at 343 and 264 nm over time.
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Light‐triggered chemical fuel generation from photolytic fuel‐carrier molecules. (a) Design and photolytic mechanism of fuel‐carrier molecules, ONB‐HFIP, which undergo UV‐triggered photolysis to release HFIP fuel and reaction byproducts. (b) Color change of ONB‐HFIP in solution as a function of UV irradiation time. (c) Time‐resolved <t>HPLC</t> chromatograms and (d) UV‐vis absorption spectra of ONB‐HFIP in solution as a function of UV irradiation time. (e) Conversion degree of photolytic reaction, estimated from the changing ratio of HPLC peak areas and UV‐vis absorption intensities at 343 and 264 nm over time.
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Light‐triggered chemical fuel generation from photolytic fuel‐carrier molecules. (a) Design and photolytic mechanism of fuel‐carrier molecules, ONB‐HFIP, which undergo UV‐triggered photolysis to release HFIP fuel and reaction byproducts. (b) Color change of ONB‐HFIP in solution as a function of UV irradiation time. (c) Time‐resolved HPLC chromatograms and (d) UV‐vis absorption spectra of ONB‐HFIP in solution as a function of UV irradiation time. (e) Conversion degree of photolytic reaction, estimated from the changing ratio of HPLC peak areas and UV‐vis absorption intensities at 343 and 264 nm over time.

Journal: Advanced Materials (Deerfield Beach, Fla.)

Article Title: Photochemical Fuel Carrier Molecules for Robotic Embodied Energy

doi: 10.1002/adma.202520447

Figure Lengend Snippet: Light‐triggered chemical fuel generation from photolytic fuel‐carrier molecules. (a) Design and photolytic mechanism of fuel‐carrier molecules, ONB‐HFIP, which undergo UV‐triggered photolysis to release HFIP fuel and reaction byproducts. (b) Color change of ONB‐HFIP in solution as a function of UV irradiation time. (c) Time‐resolved HPLC chromatograms and (d) UV‐vis absorption spectra of ONB‐HFIP in solution as a function of UV irradiation time. (e) Conversion degree of photolytic reaction, estimated from the changing ratio of HPLC peak areas and UV‐vis absorption intensities at 343 and 264 nm over time.

Article Snippet: High‐performance liquid chromatography (HPLC) spectra were obtained using an analytical reversed‐phase HPLC (Hitachi 5000 series Chromaster).

Techniques: Irradiation